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Kazuma is a former member of the Kannagi household. He was banished from the family by his father after being defeated by Ayano during the successor ceremony for Enraiha, his family's sacred sword, due to his inability to use En-Jutsu. Four years later, at the age of twenty-two, he returns to Japan as a skilled master of Fū-Jutsu.
As a Fū-Jutsushi, Kazuma's powers are extensive. Apart from being able to fly even while holding three people, Kazuma can launch blasts of wind that act as blades, and manipulate wind spirits to create a barrier, protecting his body from physical harm or reflecting light in order to camouflage himself. It has also become apparent that he possibly has the ability to manipulate electricity, given that high speed wind friction creates static electricity.
Kazuma is also a Contractor, having entered into a contract with the Kaze no Seirei-Ou, the Wind Spirit Lord. Thanks to that, Kazuma is able to draw upon all wind spirits in the atmosphere, which can amplify his powers, and allow him to heal his wounds. When using that power, his eyes turn azure blue. However, this ability puts a strain on his body. Also, when Kazuma is extremely angered, his eyes turn crimson red and his wind turns black and he is seen using mind reading powers. In this state, he has no qualms in hurting others with his abilities, as long as he gets what he wants. However, when in this state, his overall powers seem to be weaker than when he is in his regular state; when Ayano helps him snap out of his rage, he states that his black wind is pathetic.
It is later revealed that after Kazuma was banished from his family, his only desire became achieving great power. He traveled to a small town in China, where he caused all kinds of trouble. That is until he met Tsui-Ling, whom he fell in love with and eventually lived with. Kazuma no longer desired power and along with working part-time at a restaurant with her, he also took up a job as a freelancer, doing simple odd jobs. His happiness, however, came to an abrupt end when an organization used Tsui-Ling as a sacrifice to summon a powerful demon. Blaming himself for failing to protect her, Kazuma once again sought out great power, thus his making a contract with the Wind Spirit Lord. Some time after becoming a Contractor, he killed the one responsible for Tsui-Ling's death. Later, two years prior to the series' beginning, Kazuma made a name for himself as the demon-like wind mage, who did not hesitate to hurt others as long as his task was completed. However, his personality began to turn for the good once again after returning to Japan and meeting Ayano; admitting near the end of the series that he could now love another person besides Tsui-Ling.

Sixteen year old Ayano is a skilled En-Jutsushi and the successor to the Kannagi family's head. She is arrogant and irrational, usually taking action by herself even while going against orders. Though she seems undisciplined, she is very proud of her heritage. Despite claiming to hate Kazuma, Ayano develops a crush on him, but is often irritated when he makes a move on her and is prone to throwing fits of rage when he gets close to another woman. She later comes to realize that she is actually in love with him. Kazuma is also the only person she sees as stronger in power and presence than even her own father.
Ayano's power is the Crimson Flame, Kouen, although she is not yet able to consciously control it. She also holds Enraiha, the Kannagi's sacred sword, which she won by defeating Kazuma at the successor ceremony four years before the start of the story. The sword has fire properties and can be summoned by Ayano at any time. Combat-wise, Ayano tends to fight recklessly and normally her anger and pride gets the better of her. Kazuma beats her in nearly every encounter and points out the deficiences in her fighting style.

Kazuma's younger brother. He looks up to Ayano and practically worships Kazuma, stating that one day he hopes to be as strong as him so he can protect everyone. Ren has the appearance of a bishōnen, which sometimes earns him the contempt of some of his male classmates. Even so, Ren appears to be very popular at his school, excelling in his studies and in his athletic abilities. His biggest admirers include Suzuhara Kannon and Serizawa Tatsuya, who both seem to be extremely fascinated with him.
Ren later falls in love with a girl named Ayumi, only to find out that she is just a clone created to be sacrificed at a ritual. Even after saving her from the ritual, she still dies due to having a short life span, but not before she can tell him that she also loves him. Despite Ren's feelings of inadequacy early on in the series, Ayumi's death inspires Ren to become stronger so he can protect the ones he loves. Ren's power is the Golden Flame, said to have the largest purification effect.

Ren and Kazuma's strict father. Though he is responsible for banishing Kazuma from the Kannagi family, he only wanted his son to find his own path in life. Like Kazuma, Genma has trouble expressing his feelings in front of others; in fact, the both of them are so headstrong that every time they meet, they immediately break out into a destructive battle. Though Kazuma defeats him in their first battle in years, Genma is the strongest En-Jutsushi of the Kannagi's, and wields the blue Divine Flame, Souen, which only eleven others have wielded since the founding of the clan.
Despite their similarities, neither Genma nor Kazuma are willing to admit the similarities they have with each other.
Like many members of the Kannagi, Genma looks down of the Fūga Clan and wind users in general. When Kazuma goes berserk at the end of the series, Genma is the first to volunteer to assassinate his disinherited son.

Ayano's father and Genma's cousin. He is the current head of the Kannagi family. Jūgo worries about his headstrong daughter. Contrary to the Kannagi doctrine that is based solely on strength, Jūgo has been trying to stop discrimination against the Fūga Clan. He also regrets not being able to stop Kazuma's expulsion from the family. Believing that Kazuma is essential to the Kannagis, he constantly creates situations in which Ayano can form a relationship with Kazuma. As the head of the Kannagi family, Jūgo is responsible for directing the others member of the head family and branch families as well as the Fūga Clan. Jūgo is never seen in the series leaving the Kannagi compound, and rarely even leaves his meeting room.

A detective working for the Tokyo MPD's Special Investigation Unit, in charge of investigating crimes related to jutsu. She occasionally works together with Kazuma. Her department aims to become the new partner of the Kannagi family, filling the gap made by the Fūga Clan's betrayal. To that end, they assist the Ōgamis by investigating and tracking other users of jutsu. She is later revealed to be an Onmyōji, a practitioner of the Yin Yang arts who can cast spells through chants and charms. It is revealed that she had met Kazuma two years prior and that after he left, she had wished that she would never see him again.

One of Ayano's best friends and classmates. Yukari, along with Nanase, often teases Ayano about her apparent crush on Kazuma. She is well-connected to the information network of the student body and often knows what is happening around the school. Yukari's information extends beyond the school and into many areas of the Tokyo metropolis. She also carries a taser of unexplained origin with her.

One of Ayano's best friends and classmates. She and Yukari know about the existence of jutsushi. Nanase is also a very athletic student, who is part of many of their school's athletic clubs, and is admired by many of the female students. While she is not as well connected as Yukari, Nanase is just as caring and carries much sway with the students.

A member of the Kannagi, Takeya is part of the party initially sent to bring in Kazuma for questioning. He is killed in the first episode by Ryūya after being knocked down by Kazuma. He was considered to be a powerful fire user by the family, but he was unprepared for Kazuma. Takeya always acts with a calm and level head.

Sister of Takeya, who was the only person kind to her. Although a kind person at heart, having saved Kazuma from bullying ten years ago, Misao blames Kazuma for her brother's death and attempts to kill him. Her attempts fail, and she becomes a pawn in Michael's plan to take Kazuma down. In the end, Kazuma convinces her to atone for her sins by living on, and she is later instructed by Jūgo to retire to a convent.

The girl Kazuma could not protect. She was sacrificed by a member of the Armagest (possibly Bernhardt Rhodes master) to summon a demon. Rhodes then used a spell to gather her remaining essence into a being called Lapis. Before her sacrifice, she and Kazuma worked in a restaurant, and were in love. According to Lapis in the last episode, her last thoughts were "Kazuma, I want to kill you." Whether this is true or lies meant to cause Kazuma pain is unknown(Tsui-Ling may have said this out of spite towards Kazuma for being unable to save her). As Lapis, she is trained in anti-mage fighting.

A member of an American family of En-Jutsushi, specially skilled in creating and controlling spirit beasts to harness flames. She manipulates myriads of spirits into a single virtual persona to grasp tremendous power. While seemingly capable of creating different spirit beasts, her favorite is Metatron, an angel-like statue equipped with a sword. Kazuma has observed and mentioned that her fighting style is similar to Ayano's, referring to their simplistic and direct attacks, which lack any strategy or tactics. A rival against Ayano in both En-Jutsushi and Kazuma's "love."

Despite the fact that he appears to be a bishōnen of similar age to Ren, and his self-acclaim of being a Taoist-in-training, he is, in reality, a Taoist immortal whose age is measured in centuries. Lonyue came to Japan to retrieve artifacts stolen from his master, befriending Ren along the way. After recovering the lost artifacts, he opted to stay in Japan because he was bored. Lonyue, like Kazuma, teases and manipulates others in order to accomplish his goals.
Lonyue has the ability to control and manipulate his surroundings at will due his mastery of the way of Tao. His true powers are never shown, but Kazuma is revealed to have a genuine fear of fighting Lonyue again, as Lonyue was the first one Kazuma lost to in a fight since his training; even after becoming a Contractor, Kazuma is not confident in winning against him.

Son of Hyoue Kazamaki, leader of the Fūga Clan, which served the Kannagi for the last 300 years. In an elaborate plot to release the Fūga Clan's ancient master and take revenge on the Kannagi for the humiliation received since then, Ryūya's body becomes the host for a powerful yoma. Later on, he is killed in a joint attack by Kazuma and Ayano.

A young boy from the Stars of Sagacity, an organization related to Kazuma's past and Tsui-Ling's death. He uses Misao's anger at Kazuma and promised to grant her wishes. In truth, he only uses her as a medium, in order to obtain enough yoki, or life energy, to kill Kazuma. He is killed by Ayano's Shinen-empowered Enraiha.

The chairman of Armagest, a powerful organization of modern magic users. He holds a grudge against Kazuma for killing his master.

The entity that was made in Tsui-Ling's image by Burnhart. Lapis carries a crystal broad sword, but wields it with ease, and is able to match Ayano in a sword duel. It is revealed in episode 21 of the anime that Lapis has a heart, so she can feel the joy in hurting others, among other emotions.