I love most animes on crunchyroll and i think crunchyroll is the best place for you if your looking for a new anime to watch.Even though the videos arent made early like on veoh and watchanimenow crunchyroll is an excellent place to start looking for new animes to watch.

well i have a lot of favorite anime but starting from the ones i can think of from the top of my head these are my faves:

My current most favorited anime is........

Full Metal Alchemist


Darker Than Black

D.Gray Man

Vampire Knight
Vampire Knight Guilty

Zero no Tsukaima
Zero no Tsukaima : Futatsuki no Kishi
Zero no Tsukaima : Princess no Rondo

Bleach

Code Geass : Lelouch of the Rebellion
Code Geass R2

Shugo Chara

Good Witch of West

Beating Angel Dokuro Chan

BLASSREITER

Tower of Druaga : The Aegis of URUK

Sekirei

Natsume Yuujinchou

Xamd Lost Memories

Toradora

Time of Eve

Tales of the Abyss

Soul Eater

Ouran High School Host Club

Kuroshitsuji

Digimon Adventure 02